Yr Athro Serena Margadonna

Cadair

Chemical Engineering

s.margadonna@abertawe.ac.uk

405
Pedwerydd Llawr
Adeilad Gogleddol Peirianneg
Campws y Bae

Ar gael ar gyfer Goruchwyliaeth Ôl-raddedig

Dolenni Ymchwil

https://orcid.org/0000-0002-6996-6562

Trosolwg

Yn ddiweddar, penodwyd yr Athro Margadonna yn Gadair ym Mheirianneg Deunyddiau.

Ysbrydolwyd ei gwaith wrth iddi sylweddoli bod prif ddatblygiadau technoleg fodern yn dibynnu’n llwyr ar argaeledd deunyddiau sydd yn cynnwys nifer o swyddogaethau ac yn medru gweithredu ar raddfeydd o hyd gwahanol, mewn amodau caled fel eithafion pwysedd/tymheredd ac amgylcheddau cyrydol iawn. Mae’r gofynion perfformio ar gyfer deunyddiau yn gynyddol ddyrys ac yn gofyn am ymchwil gwirioneddol rhyngddisgyblaethol.

Dros y blynyddoedd mae’r Athro Margadonna wedi casglu gwybodaeth a dod i ddeall nifer o feysydd gwyddonol gwahanol gan ddechrau gyda’i chefndir mewn cemeg, anhepgor am ddylunio a chynhyrchu deunyddiau newydd, drwy ffiseg sylwedd dwys a pheirianneg broses. Cyflawnwyd hyn drwy weithio mewn nifer o sefydliadau academaidd ac ymweld â nifer o labordai rhyngwladol sydd wedi arwain at sefydlu cysylltiadau a chydweithio gyda gwyddonwyr blaenllaw ledled y byd. Mae ei hagwedd ryngddisgyblaethol wedi cynhyrchu nifer o ddatblygiadau arwyddocaol sydd wedi denu cydnabyddiaeth gan gyfoedion fel y gwelir mewn nifer o gyhoeddiadau proffil uchel a gwobrau rhyngwladol.

Mae ymchwil presennol yr Athro Margadonna’n canolbwyntio ar ddeunyddiau a phrosesau technolegau sydd oll yn ymwneud â chludo, storio a chynhyrchu ynni. Ei gweledigaeth yw cyfrannu at yr her ynni fyd-eang gan ddatblygu datrysiadau sy’n gost-effeithiol ac yn gynaliadwy’n amgylcheddol.

Cyhoeddiadau

Uchafbwyntiau Ymchwil

Aupama, V., Sangsawang, J., Kao-ian, W., Wannapaiboon, S., Pimoei, J., yoopensuk, W., Opchoei, M., Tehrani, Z., Margadonna, S., & Kheawhom, S. (2024). Adaptive COF-PVDF composite artificial solid electrolyte interphase for stable aqueous zinc batteries. Electrochimica Acta, 506, 145059
https://doi.org/10.1016/j.electacta.2024.145059, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa67929
Willow, A., Hussein, H., Vajirakaphan, S., Chasri, A., & Margadonna, S. (2022). Improving In-Situ Sodium Metal Plating on Copper Foil Through Optimization of Mechanical Pressure: Towards High-Performance Anode-Free Sodium Ion Batteries. Frontiers in Energy Research, 10
https://doi.org/10.3389/fenrg.2022.888321, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa59757
Worsley, E., Margadonna, S., & Bertoncello, P. (2022). Application of Graphene Nanoplatelets in Supercapacitor Devices: A Review of Recent Developments. Nanomaterials, 12(20), 3600
https://doi.org/10.3390/nano12203600, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa61568
Romani, L., Speltini, A., Ambrosio, F., Mosconi, E., Profumo, A., Marelli, M., Margadonna, S., Milella, A., Fracassi, F., Listorti, A., Angelis, F., & Malavasi, L. (2021). Water‐Stable DMASnBr3 Lead‐Free Perovskite for Effective Solar‐Driven Photocatalysis. Angewandte Chemie, 133(7), 3655-3662.
https://doi.org/10.1002/ange.202007584, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa55528
Yusenko, K., Sottmann, J., Emerich, H., Crichton, W., Malavasi, L., & Margadonna, S. (2015). Hyper-expanded interlayer separations in superconducting barium intercalates of FeSe. Chem. Commun., 51(33), 7112-7115.
https://doi.org/10.1039/C5CC01583A, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa20488
http://pubs.rsc.org/en/content/articlelanding/2015/cc/c5cc01583a#!divAbstract
Sottmann, J., Bernal, F., Yusenko, K., Herrmann, M., Emerich, H., Wragg, D., & Margadonna, S. (2016). In operando Synchrotron XRD/XAS Investigation of Sodium Insertion into the Prussian Blue Analogue Cathode Material Na 1.32 Mn[Fe(CN) 6 ] 0.83 · z H 2 O. Electrochimica Acta, 200, 305-313.
https://doi.org/10.1016/j.electacta.2016.03.131, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa26940
Nakagawa, T., Yuan, Z., Zhang, J., Yusenko, K., Drathen, C., Liu, Q., Margadonna, S., & Jin, C. (2016). Structure and magnetic property of potassium intercalated pentacene: observation of superconducting phase in KxC22H14. Journal of Physics: Condensed Matter, 28(48), 484001
https://doi.org/10.1088/0953-8984/28/48/484001, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa30247
Yusenko, K., Bykova, E., Bykov, M., Gromilov, S., Kurnosov, A., Prescher, C., Prakapenka, V., Crichton, W., Hanfland, M., Margadonna, S., & Dubrovinsky, L. (2017). High-pressure high-temperature stability of hcp-IrxOs1−x (x = 0.50 and 0.55) alloys. Journal of Alloys and Compounds, 700, 198-207.
https://doi.org/10.1016/j.jallcom.2016.12.207, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa31566
Jones, D., Gomez, V., Bear, J., Rome, B., Mazzali, F., McGettrick, J., Lewis, A., Margadonna, S., Al-Masry, W., & Dunnill, C. (2017). Active removal of waste dye pollutants using Ta3N5/W18O49 nanocomposite fibres. Scientific Reports, 7(1)
https://doi.org/10.1038/s41598-017-04240-4, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa34442
Jalalian-Khakshour, A., Phillips, C., Jackson, L., Dunlop, T., Margadonna, S., & Deganello, D. (2019). Solid-state synthesis of NASICON (Na3Zr2Si2PO12) using nanoparticle precursors for optimisation of ionic conductivity. Journal of Materials Science, 55, 2291-2302.
https://doi.org/10.1007/s10853-019-04162-8, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa52708
Mazzali, F., Orzech, M., Adomkevicius, A., Pisanu, A., Malavasi, L., Deganello, D., & Margadonna, S. (2019). Designing a High-Power Sodium-Ion Battery by in Situ Metal Plating. ACS Applied Energy Materials, 2(1), 344-353.
https://doi.org/10.1021/acsaem.8b01361, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa48051
Povia, M., Sottmann, J., Portale, G., Knudsen, K., Margadonna, S., & Sartori, S. (2018). Operando SAXS/WAXS on the a-P/C as the Anode for Na-Ion Batteries. The Journal of Physical Chemistry C, 122(11), 5917-5923.
https://doi.org/10.1021/acs.jpcc.7b12825, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa38963
Yusenko, K., Riva, S., Crichton, W., Spektor, K., Bykova, E., Pakhomova, A., Tudball, A., Kupenko, I., Rohrbach, A., Klemme, S., Mazzali, F., Margadonna, S., Lavery, N., & Brown, S. (2018). High-pressure high-temperature tailoring of High Entropy Alloys for extreme environments. Journal of Alloys and Compounds, 738, 491-500.
https://doi.org/10.1016/j.jallcom.2017.12.216, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa37789
Orzech, M., Mazzali, F., McGettrick, J., Pleydell-Pearce, C., Watson, T., Voice, W., Jarvis, D., & Margadonna, S. (2017). Synergic effect of Bi, Sb and Te for the increased stability of bulk alloying anodes for sodium-ion batteries. Journal of Materials Chemistry A, 5(44), 23198-23208.
https://doi.org/10.1039/C7TA07648G, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa36243
Sottmann, J., Di Michiel, M., Fjellvåg, H., Malavasi, L., Margadonna, S., Vajeeston, P., Vaughan, G., & Wragg, D. (2017). Chemical Structures of Specific Sodium Ion Battery Components Determined by Operando Pair Distribution Function and X-ray Diffraction Computed Tomography. Angewandte Chemie International Edition, 56(38), 11385-11389.
https://doi.org/10.1002/anie.201704271, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa34514
http://onlinelibrary.wiley.com/doi/10.1002/anie.201704271/epdf
Sottmann, J., Homs-Regojo, R., Wragg, D., Fjellvåg, H., Margadonna, S., & Emerich, H. (2016). Versatile electrochemical cell for Li/Na-ion batteries and high-throughput setup for combined operando X-ray diffraction and absorption spectroscopy. Journal of Applied Crystallography, 49(6), 1972-1981.
https://doi.org/10.1107/S160057671601428X, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa31079
https://doi.org/10.1107/S160057671601428X
Samarasingha, P., Sottmann, J., Margadonna, S., Emerich, H., Nilsen, O., & Fjellvåg, H. (2016). In situ synchrotron study of ordered and disordered LiMn1.5Ni0.5O4 as lithium ion battery positive electrode. Acta Materialia, 116, 290-297.
https://doi.org/10.1016/j.actamat.2016.06.040, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa29192
Crichton, W., Yusenko, K., Riva, S., Mazzali, F., & Margadonna, S. (2016). An Alternative Route to Pentavalent Postperovskite. Inorganic Chemistry, 55(12), 5738-5740.
https://doi.org/10.1021/acs.inorgchem.6b00780, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa28821
Yusenko, K., Bykova, E., Bykov, M., Gromilov, S., Kurnosov, A., Prescher, C., Prakapenka, V., Hanfland, M., van Smaalen, S., Margadonna, S., & Dubrovinsky, L. (2014). Compressibility of Ir–Os alloys under high pressure. Journal of Alloys and Compounds, 622, 155-161.
https://doi.org/10.1016/j.jallcom.2014.09.210, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa21221
Margadonna, S. (2016). Observation of Sb2S3-type post-post-perovskite in NaFeF3. Implications for ABX3 and A2X3 systems at ultrahigh pressure. Mineralogical Magazine, 80(4), 659-674.
https://doi.org/10.1180/minmag.2016.080.017, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa29037
http://minmag.geoscienceworld.org/content/80/4/659.full.pdf+html

Holl Ymchwil

Erthyglau Cylchgronau

Aupama, V., Sangsawang, J., Kao-ian, W., Wannapaiboon, S., Pimoei, J., yoopensuk, W., Opchoei, M., Tehrani, Z., Margadonna, S., & Kheawhom, S. (2024). Adaptive COF-PVDF composite artificial solid electrolyte interphase for stable aqueous zinc batteries. Electrochimica Acta, 506, 145059
https://doi.org/10.1016/j.electacta.2024.145059, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa67929
Worsley, E., Margadonna, S., & Bertoncello, P. (2022). Application of Graphene Nanoplatelets in Supercapacitor Devices: A Review of Recent Developments. Nanomaterials, 12(20), 3600
https://doi.org/10.3390/nano12203600, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa61568
Willow, A., Hussein, H., Vajirakaphan, S., Chasri, A., & Margadonna, S. (2022). Improving In-Situ Sodium Metal Plating on Copper Foil Through Optimization of Mechanical Pressure: Towards High-Performance Anode-Free Sodium Ion Batteries. Frontiers in Energy Research, 10
https://doi.org/10.3389/fenrg.2022.888321, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa59757
Romani, L., Speltini, A., Ambrosio, F., Mosconi, E., Profumo, A., Marelli, M., Margadonna, S., Milella, A., Fracassi, F., Listorti, A., Angelis, F., & Malavasi, L. (2021). Water‐Stable DMASnBr3 Lead‐Free Perovskite for Effective Solar‐Driven Photocatalysis. Angewandte Chemie, 133(7), 3655-3662.
https://doi.org/10.1002/ange.202007584, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa55528
Jalalian-Khakshour, A., Phillips, C., Jackson, L., Dunlop, T., Margadonna, S., & Deganello, D. (2019). Solid-state synthesis of NASICON (Na3Zr2Si2PO12) using nanoparticle precursors for optimisation of ionic conductivity. Journal of Materials Science, 55, 2291-2302.
https://doi.org/10.1007/s10853-019-04162-8, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa52708
Mazzali, F., Orzech, M., Adomkevicius, A., Pisanu, A., Malavasi, L., Deganello, D., & Margadonna, S. (2019). Designing a High-Power Sodium-Ion Battery by in Situ Metal Plating. ACS Applied Energy Materials, 2(1), 344-353.
https://doi.org/10.1021/acsaem.8b01361, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa48051
Yusenko, K., Riva, S., Crichton, W., Spektor, K., Bykova, E., Pakhomova, A., Tudball, A., Kupenko, I., Rohrbach, A., Klemme, S., Mazzali, F., Margadonna, S., Lavery, N., & Brown, S. (2018). High-pressure high-temperature tailoring of High Entropy Alloys for extreme environments. Journal of Alloys and Compounds, 738, 491-500.
https://doi.org/10.1016/j.jallcom.2017.12.216, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa37789
Povia, M., Sottmann, J., Portale, G., Knudsen, K., Margadonna, S., & Sartori, S. (2018). Operando SAXS/WAXS on the a-P/C as the Anode for Na-Ion Batteries. The Journal of Physical Chemistry C, 122(11), 5917-5923.
https://doi.org/10.1021/acs.jpcc.7b12825, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa38963
Jones, D., Gomez, V., Bear, J., Rome, B., Mazzali, F., McGettrick, J., Lewis, A., Margadonna, S., Al-Masry, W., & Dunnill, C. (2017). Active removal of waste dye pollutants using Ta3N5/W18O49 nanocomposite fibres. Scientific Reports, 7(1)
https://doi.org/10.1038/s41598-017-04240-4, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa34442
Orzech, M., Mazzali, F., McGettrick, J., Pleydell-Pearce, C., Watson, T., Voice, W., Jarvis, D., & Margadonna, S. (2017). Synergic effect of Bi, Sb and Te for the increased stability of bulk alloying anodes for sodium-ion batteries. Journal of Materials Chemistry A, 5(44), 23198-23208.
https://doi.org/10.1039/C7TA07648G, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa36243
Sottmann, J., Di Michiel, M., Fjellvåg, H., Malavasi, L., Margadonna, S., Vajeeston, P., Vaughan, G., & Wragg, D. (2017). Chemical Structures of Specific Sodium Ion Battery Components Determined by Operando Pair Distribution Function and X-ray Diffraction Computed Tomography. Angewandte Chemie International Edition, 56(38), 11385-11389.
https://doi.org/10.1002/anie.201704271, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa34514
http://onlinelibrary.wiley.com/doi/10.1002/anie.201704271/epdf
Yusenko, K., Bykova, E., Bykov, M., Gromilov, S., Kurnosov, A., Prescher, C., Prakapenka, V., Crichton, W., Hanfland, M., Margadonna, S., & Dubrovinsky, L. (2017). High-pressure high-temperature stability of hcp-IrxOs1−x (x = 0.50 and 0.55) alloys. Journal of Alloys and Compounds, 700, 198-207.
https://doi.org/10.1016/j.jallcom.2016.12.207, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa31566
Sottmann, J., Homs-Regojo, R., Wragg, D., Fjellvåg, H., Margadonna, S., & Emerich, H. (2016). Versatile electrochemical cell for Li/Na-ion batteries and high-throughput setup for combined operando X-ray diffraction and absorption spectroscopy. Journal of Applied Crystallography, 49(6), 1972-1981.
https://doi.org/10.1107/S160057671601428X, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa31079
https://doi.org/10.1107/S160057671601428X
Crichton, W., Yusenko, K., Riva, S., Mazzali, F., & Margadonna, S. (2016). An Alternative Route to Pentavalent Postperovskite. Inorganic Chemistry, 55(12), 5738-5740.
https://doi.org/10.1021/acs.inorgchem.6b00780, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa28821
Nakagawa, T., Yuan, Z., Zhang, J., Yusenko, K., Drathen, C., Liu, Q., Margadonna, S., & Jin, C. (2016). Structure and magnetic property of potassium intercalated pentacene: observation of superconducting phase in KxC22H14. Journal of Physics: Condensed Matter, 28(48), 484001
https://doi.org/10.1088/0953-8984/28/48/484001, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa30247
Samarasingha, P., Sottmann, J., Margadonna, S., Emerich, H., Nilsen, O., & Fjellvåg, H. (2016). In situ synchrotron study of ordered and disordered LiMn1.5Ni0.5O4 as lithium ion battery positive electrode. Acta Materialia, 116, 290-297.
https://doi.org/10.1016/j.actamat.2016.06.040, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa29192
Margadonna, S. (2016). Observation of Sb2S3-type post-post-perovskite in NaFeF3. Implications for ABX3 and A2X3 systems at ultrahigh pressure. Mineralogical Magazine, 80(4), 659-674.
https://doi.org/10.1180/minmag.2016.080.017, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa29037
http://minmag.geoscienceworld.org/content/80/4/659.full.pdf+html
Sottmann, J., Bernal, F., Yusenko, K., Herrmann, M., Emerich, H., Wragg, D., & Margadonna, S. (2016). In operando Synchrotron XRD/XAS Investigation of Sodium Insertion into the Prussian Blue Analogue Cathode Material Na 1.32 Mn[Fe(CN) 6 ] 0.83 · z H 2 O. Electrochimica Acta, 200, 305-313.
https://doi.org/10.1016/j.electacta.2016.03.131, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa26940
Yusenko, K., Sottmann, J., Emerich, H., Crichton, W., Malavasi, L., & Margadonna, S. (2015). Hyper-expanded interlayer separations in superconducting barium intercalates of FeSe. Chem. Commun., 51(33), 7112-7115.
https://doi.org/10.1039/C5CC01583A, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa20488
http://pubs.rsc.org/en/content/articlelanding/2015/cc/c5cc01583a#!divAbstract
Yusenko, K., Bykova, E., Bykov, M., Gromilov, S., Kurnosov, A., Prescher, C., Prakapenka, V., Hanfland, M., van Smaalen, S., Margadonna, S., & Dubrovinsky, L. (2014). Compressibility of Ir–Os alloys under high pressure. Journal of Alloys and Compounds, 622, 155-161.
https://doi.org/10.1016/j.jallcom.2014.09.210, SU Repository: https://cronfa.swan.ac.uk/Record/cronfa21221

Goruchwyliaeth

Automotive Batteries- Sodium-ion and Lithium-ion Unified Technology (cyfredol)

PhD

Goruchwyliwr arall: Prof Antonio Gil
Efficient direct recycling of spent Li-ion battery cathodes (cyfredol)

PhD

Goruchwyliwr arall: Dr Zari Tehrani
High performance carbon anodes for asymmetric supercapacitors (cyfredol)

PhD

Goruchwyliwr arall: Prof Davide Deganello
Synthesis and Surface functionalisation of TiO2 nanoparticles - Development of versatile colloidal formulations for the fabrication of photocatalytic self-cleaning glass. (cyfredol)

PhD

Goruchwyliwr arall: Dr Charlie Dunnill
Synthesis of Solid-state NASICON Electrolytes for Sodium-ion Batteries (cyfredol)

PhD

Goruchwyliwr arall: Dr Jenny Baker
Development of Sodium Solid-State Electrolytes for SolidState batteries (cyfredol)

PhD

Goruchwyliwr arall: Dr Anji Munnangi
Hard Carbon and Sodium Rhodizonate Electrodes for Sodium-Ion Batteries (dyfarnwyd 2024)

PhD

Goruchwyliwr arall: Prof Davide Deganello
Synthesis and Characterization of Sodium Rich cathodes for next-generation sustainable batteries (cyfredol)

EngD

Goruchwyliwr arall: Prof Davide Deganello
Development of greener electrode coatings for next generation supercapacitors (cyfredol)

EngD

Goruchwyliwr arall: Dr Paolo Bertoncello
Molecular Vapor Deposition for Next Generation Functional«br /» Coatings«br /» (cyfredol)

EngD

Goruchwyliwr arall: Prof Owen Guy

Yr Athro Serena Margadonna

Cyfeiriad ebost

Dolenni Ymchwil

Trosolwg

Cyhoeddiadau

Uchafbwyntiau Ymchwil

Holl Ymchwil

Erthyglau Cylchgronau

Goruchwyliaeth

Automotive Batteries- Sodium-ion and Lithium-ion Unified Technology (cyfredol)

Efficient direct recycling of spent Li-ion battery cathodes (cyfredol)

High performance carbon anodes for asymmetric supercapacitors (cyfredol)

Synthesis and Surface functionalisation of TiO2 nanoparticles - Development of versatile colloidal formulations for the fabrication of photocatalytic self-cleaning glass. (cyfredol)

Synthesis of Solid-state NASICON Electrolytes for Sodium-ion Batteries (cyfredol)

Development of Sodium Solid-State Electrolytes for SolidState batteries (cyfredol)

Hard Carbon and Sodium Rhodizonate Electrodes for Sodium-Ion Batteries (dyfarnwyd 2024)

Synthesis and Characterization of Sodium Rich cathodes for next-generation sustainable batteries (cyfredol)

Development of greener electrode coatings for next generation supercapacitors (cyfredol)

Molecular Vapor Deposition for Next Generation Functional«br /» Coatings«br /» (cyfredol)